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Proceedings Paper

Self-consistent modeling of photoionization and the Kerr effect in bulk solids
Author(s): Jeremy R. Gulley; Thomas E Lanier
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Paper Abstract

In calculations of ultrafast laser-induced ionization the treatment of fundamental mechanisms such as photoionization and the Kerr effect are treated in isolation using monochromatic perturbative approaches. Such approaches are often questionable for pulses of ultrashort duration and multi-chromatic spectra. In this work we address this issue by solving the quantum optical Bloch equations in a 3D quasi-momentum space and show how to couple this model to ultrashort pulse propagation in dielectrics. This approach self-consistently couples a quantum calculation of the photoionization yield, the photoionization current, and the current from free-carriers with the traditional Kerr effect (self-focusing and self phase modulation) without resort to a perturbative treatment. The material band structure is taken in the tight binding limit and is periodic in the crystal momentum space. As this model makes no assumption about the pulse spectrum, we examine the laser-material interaction of strongly chirped pulses and multi-color multi-pulse schemes of laser-induced material modification. These results are compared to those predicted by standard treatments, such as the Keldysh model of photoionization, for pulses of ultrashort duration.

Paper Details

Date Published: 23 November 2015
PDF: 7 pages
Proc. SPIE 9632, Laser-Induced Damage in Optical Materials: 2015, 96320X (23 November 2015); doi: 10.1117/12.2195293
Show Author Affiliations
Jeremy R. Gulley, Kennesaw State Univ. (United States)
Thomas E Lanier, Kennesaw State Univ. (United States)

Published in SPIE Proceedings Vol. 9632:
Laser-Induced Damage in Optical Materials: 2015
Gregory J. Exarhos; Vitaly E. Gruzdev; Joseph A. Menapace; Detlev Ristau; MJ Soileau, Editor(s)

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